Titre | Infrared spectra of the one-dimensional quarter-filled Wigner lattice compounds delta-(EDT-TTF-CONMe2)(2)X (X = AsF6, Br): Domain-wall excitations |
Type de publication | Article de revue |
Auteur | Antal, Ágnes, Knoblauch, T., Dressel, Martin, Batail, Patrick , Drichko, Natalia |
Type | Article scientifique dans une revue à comité de lecture |
Année | 2013 |
Langue | Anglais |
Date | 02/2013 |
Numéro | 7 |
Volume | 87 |
Titre de la revue | Physical Review B |
ISSN | 1098-0121 |
Mots-clés | organic conductors |
Résumé en anglais | Optical investigations of quarter-filled charge ordered insulators delta-(EDT-TTF-CONMe2)(2)X, X = AsF6, Br are reported. The spectra evidence the one-dimensional nature of the systems at all temperatures. The charge order exists already at room temperature, the optical gap is estimated to be of the order of 550 cm(-1) for the X = Br compound and about 700 cm(-1) for the X = AsF6 material. The optical response in the direction of the stacks is discussed in terms of domain-wall excitations of one-dimensional quarter-filled Wigner lattice at moderate values of nearest-neighbor electronic repulsion. A similarity between the effects of temperature contraction and chemical pressure is found. |
URL de la notice | http://okina.univ-angers.fr/publications/ua2672 |
DOI | 10.1103/PhysRevB.87.075118 |